Enhancing catalytic amine regeneration in CO2 capture using ZrOxHy-coated mesoporous silica

Zhou, Cheng;Shao, Yuewen;Beydokhti, Mostafa Torka;Ma, Jing;Sels, Bert F.;et.al.
(2026) Chemical Communications — Vol. 62, n° 27, p. 7198-7201 (2026)

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Authors
  • Zhou, Chengorcid-logoCenter for Sustainable Catalysis and Engineering, KU Leuven, Celestijnenlaan 200F, Heverlee 3001, Belgium
    Author
  • Shao, YuewenCenter for Sustainable Catalysis and Engineering, KU Leuven, Celestijnenlaan 200F, Heverlee 3001, Belgium
    Author
  • Beydokhti, Mostafa Torkaorcid-logoCenter for Sustainable Catalysis and Engineering, KU Leuven, Celestijnenlaan 200F, Heverlee 3001, Belgium
    Author
  • Ma, JingCenter for Sustainable Catalysis and Engineering, KU Leuven, Celestijnenlaan 200F, Heverlee 3001, Belgium
    Author
  • Eloy, PierreUCLouvain
    Author
  • Author
  • Sels, Bert F.orcid-logoCenter for Sustainable Catalysis and Engineering, KU Leuven, Celestijnenlaan 200F, Heverlee 3001, Belgium
    Author
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Abstract
Bulk ZrOxHy is an effective catalyst for amine regeneration in CO2 absorption, but its high cost and poor support stability may hinder application. Here, ZrOxHy is deposited as a theoratical monolayer within MCM-41 mesopores, achieving similar stable catalytic activity to bulk ZrOxHy with just 13 wt% Zr loading, offering a cost-effective path toward industrial use.
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Citations

Zhou, C., Shao, Y., Beydokhti, M. T., Ma, J., Eloy, P., Debecker, D., Dusselier, M., Vermeiren, W., & Sels, B. F. (2026). Enhancing catalytic amine regeneration in CO2 capture using ZrOxHy-coated mesoporous silica. Chemical Communications, 62(27), 7198-7201. https://doi.org/10.1039/d5cc06632h (Original work published 2026)