Increased Catalytic Activity of Surface-Immobilized Palladium Complexes in the Fluorogenic Deprotection of an Alloc-Derivatized Coumarin

Fernandes, Antony;Hensenne, Peter;Mathy, Bertrand;Guo, Weiming;Riant, Olivier;et.al.
(2012) Chemistry: A European Journal — Vol. 18, n° 3, p. 788-792 (2012)

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Abstract
Catalytic surfaces have been prepared by complexation of palladium on self-assembled terpyridine monolayers on silicon. A reaction-based fluorogenic probe was developed to allow facile visualization of the catalytic potential of the surface (see figure). Superior activity of the immobilized catalyst compared with the homogeneous control reactions is demonstrated.
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Fernandes, A., Hensenne, P., Mathy, B., Guo, W., Nysten, B., Jonas, A., & Riant, O. (2012). Increased Catalytic Activity of Surface-Immobilized Palladium Complexes in the Fluorogenic Deprotection of an Alloc-Derivatized Coumarin. Chemistry: A European Journal, 18(3), 788-792. https://doi.org/10.1002/chem.201102245 (Original work published 2012)