One “Click” to controlled bifunctional supported catalysts for the Cu/TEMPO-catalyzed aerobic oxidation of alcohols

Fernandes, Antony; Riant, Olivier; Jonas, Alain; Jensen, Klavs F.

doi:10.1039/c6ra05026c

One “Click” to controlled bifunctional supported catalysts for the Cu/TEMPO-catalyzed aerobic oxidation of alcohols

Fernandes, Antony

;

Riant, Olivier

;

Jonas, Alain

;

Jensen, Klavs F.

(2016) RSC Advances — Vol. 6, p. 36602-36605 (2016)

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Authors

Fernandes, AntonyUCLouvain
Author
Riant, OlivierUCLouvain
Author
Jonas, AlainUCLouvain
Author
Jensen, Klavs F.Massachusett Instutute of Technology, USA
Author

Abstract

A simple and reliable methodology is described for the preparation of heterogeneous bifunctional catalysts with a high control over surface composition. The strategy relies on the grafting of a mix of catalytic components from an azide-functionalized silica platform using the CuAAC reaction. The resulting finely engineered supported catalysts are employed in the model Cu/TEMPO-catalyzed aerobic oxidation of benzylic alcohol.

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Fernandes, A., Riant, O., Jonas, A., & Jensen, K. F. (2016). One “Click” to controlled bifunctional supported catalysts for the Cu/TEMPO-catalyzed aerobic oxidation of alcohols. RSC Advances, 6, 36602-36605. https://doi.org/10.1039/c6ra05026c (Original work published 2016)